Abstract
Background: Due to its high toxicity and bioaccumulation, the existence of mercury in the environment is always a big threat to human beings. In order to control mercury pollution, scientists have put great efforts in the past decades.
Methods: Precipitation, adsorption, membrane separation, biological treatment and ion exchange are reviewed as a remover for mercury removal. For each material type, we not only reported on the removal mechanism, but also discussed the best areas for it. The correlation method and step-to-step focusing method have been used for references.
Results: For better mercury removal, the ways above are compared together. The mechanisms of removing mercury in different ways are summarized in this paper.
Conclusion: With the exploration and application of research, people have mastered a variety of mature technologies for the treatment of mercury-containing wastewater. Using inexpensive adsorbents is a cost-effective method for treating low concentrations of heavy metal wastewater. Ion exchange with a fast removal rate has been widely used in the field of heavy metal removal from wastewater. The biological treatment method can effectively treat low-concentration mercurycontaining wastewater. However, there is still a need to develop novel mercury removers with high capacity, fast removal rate, and low removal limit. Nanomaterials with a high specific surface area on substrate with synergistic effects, such as high adsorption and ion exchange, are the future research points.
Keywords: Mercury, removal, method, wastewater, nanomaterial, mechanism.
Graphical Abstract
[http://dx.doi.org/10.1155/2015/372459] [PMID: 26236539]
[http://dx.doi.org/10.1038/s41467-018-07300-z] [PMID: 30451827]
[http://dx.doi.org/10.1016/j.ccr.2016.10.009]
[http://dx.doi.org/10.1016/S0048-9697(03)00135-9] [PMID: 12826386]
[http://dx.doi.org/10.1080/10408440600845619] [PMID: 16973445]
[http://dx.doi.org/10.1289/ehp.9310031] [PMID: 8354179]
[http://dx.doi.org/10.1016/j.autrev.2016.09.020] [PMID: 27666813]
[http://dx.doi.org/10.1080/20016491089226]
[http://dx.doi.org/10.1016/j.neuro.2016.04.010] [PMID: 27090823]
[http://dx.doi.org/10.1002/jat.3151] [PMID: 25854323]
[http://dx.doi.org/10.1039/C5EM00561B] [PMID: 26745831]
[http://dx.doi.org/10.3390/ijms17030361] [PMID: 26978352]
[http://dx.doi.org/10.1016/j.marchem.2016.07.002]
[http://dx.doi.org/10.1016/j.envpol.2017.05.085] [PMID: 28599207]
[http://dx.doi.org/10.1515/revac-2013-0003]
[http://dx.doi.org/10.1038/nmat1368] [PMID: 15867920]
[http://dx.doi.org/10.1002/adfm.201606572]
[http://dx.doi.org/10.1007/s10311-016-0595-x]
[http://dx.doi.org/10.1016/j.jhazmat.2008.01.006] [PMID: 18280650]
[http://dx.doi.org/10.1080/09593330309385626] [PMID: 12916841]
[http://dx.doi.org/10.1016/j.fuel.2009.10.031]
[http://dx.doi.org/10.1016/j.cej.2018.03.126]
[http://dx.doi.org/10.1016/j.molliq.2018.05.048]
[http://dx.doi.org/10.1039/C7NJ00663B]
[http://dx.doi.org/10.1007/430_013]
[http://dx.doi.org/10.1016/j.jece.2014.01.004]
[http://dx.doi.org/10.1016/j.cej.2013.03.082]
[http://dx.doi.org/10.1016/j.jhazmat.2014.03.037] [PMID: 24727013]
[http://dx.doi.org/10.1201/9781351069465]
[http://dx.doi.org/10.1016/j.cej.2009.10.029]
[http://dx.doi.org/10.1016/j.jcis.2004.08.168] [PMID: 15589536]
[http://dx.doi.org/10.1016/j.watres.2004.09.027] [PMID: 15644247]
[http://dx.doi.org/10.1016/j.jhazmat.2011.07.021] [PMID: 21803490]
[http://dx.doi.org/10.1021/cm8024022]
[http://dx.doi.org/10.1016/S0043-1354(00)00044-0]
[http://dx.doi.org/10.1021/ja0506859] [PMID: 15941284]
[http://dx.doi.org/10.1089/ees.2008.0418]
[http://dx.doi.org/10.1002/adfm.200601230]
[http://dx.doi.org/10.1126/science.1142535] [PMID: 17656718]
[http://dx.doi.org/10.1021/am301031g] [PMID: 22853320]
[http://dx.doi.org/10.1016/j.apsusc.2005.11.034]
[http://dx.doi.org/10.1021/ie901194r]
[http://dx.doi.org/10.1016/j.jenvman.2018.02.052] [PMID: 29477852]
[http://dx.doi.org/10.1007/s11356-017-9086-2] [PMID: 28470495]
[http://dx.doi.org/10.1021/ic101935f] [PMID: 21082837]
[http://dx.doi.org/10.1021/ja400212k] [PMID: 23646999]
[http://dx.doi.org/10.1021/cm200557e]
[http://dx.doi.org/10.1002/chem.201403382] [PMID: 25210002]
[http://dx.doi.org/10.1021/acscentsci.7b00605] [PMID: 29632880]
[http://dx.doi.org/10.1016/j.scitotenv.2018.02.033] [PMID: 30857103]
[http://dx.doi.org/10.1007/s11814-017-0116-z]
[http://dx.doi.org/10.1007/s10098-017-1374-5]
[http://dx.doi.org/10.1039/C7NJ01450C]
[http://dx.doi.org/10.1080/09542299.2017.1378596]
[http://dx.doi.org/10.1016/j.micromeso.2018.05.038]
[http://dx.doi.org/10.1016/j.jallcom.2017.12.087]
[http://dx.doi.org/10.1016/j.biortech.2018.04.053] [PMID: 29689437]
[http://dx.doi.org/10.1007/s11164-018-3431-z]
[http://dx.doi.org/10.2166/wst.2017.165] [PMID: 28659524]
[http://dx.doi.org/10.1016/j.fuel.2017.04.105]
[http://dx.doi.org/10.1016/j.jcis.2016.10.002] [PMID: 27723483]
[http://dx.doi.org/10.1016/j.jcis.2017.05.104] [PMID: 28601744]
[http://dx.doi.org/10.1007/s11356-017-0508-y] [PMID: 29143259]
[http://dx.doi.org/10.1021/acs.iecr.7b02743]
[http://dx.doi.org/10.1021/acsami.6b15106] [PMID: 28051307]
[http://dx.doi.org/10.1016/j.cherd.2017.11.014]
[http://dx.doi.org/10.1016/j.jes.2016.12.016] [PMID: 29908736]
[http://dx.doi.org/10.1007/s13738-018-1371-6]
[http://dx.doi.org/10.1016/j.cej.2016.10.126]
[http://dx.doi.org/10.1016/j.jcis.2017.03.014] [PMID: 28314146]
[http://dx.doi.org/10.1016/j.chemosphere.2016.09.133] [PMID: 27710842]
[http://dx.doi.org/10.1007/s11356-017-8780-4] [PMID: 28337626]
[http://dx.doi.org/10.1039/C7FD00012J] [PMID: 28607993]
[http://dx.doi.org/10.1021/acssuschemeng.7b03188]
[http://dx.doi.org/10.1016/j.ijbiomac.2017.11.027] [PMID: 29126940]
[http://dx.doi.org/10.1016/j.jclepro.2018.05.043]
[http://dx.doi.org/10.1021/acs.iecr.7b03093]
[http://dx.doi.org/10.1007/s11270-017-3511-5]
[http://dx.doi.org/10.1016/j.chemosphere.2017.12.186] [PMID: 29304455]
[http://dx.doi.org/10.1016/j.ijbiomac.2018.01.206] [PMID: 29425868]
[http://dx.doi.org/10.1007/s10311-018-0746-3]
[http://dx.doi.org/10.1007/s10971-018-4723-x]
[http://dx.doi.org/10.2166/wst.2018.117] [PMID: 29698245]
[http://dx.doi.org/10.1016/j.jclepro.2018.06.027]
[http://dx.doi.org/10.1021/acs.energyfuels.7b03094]
[http://dx.doi.org/10.1007/s11164-017-3091-4]
[http://dx.doi.org/10.1002/gch2.201700078] [PMID: 31565300]
[http://dx.doi.org/10.1021/acssuschemeng.7b03040]
[http://dx.doi.org/10.1002/slct.201702851]
[http://dx.doi.org/10.1016/j.cej.2017.04.005]
[http://dx.doi.org/10.1007/s10971-017-4362-7]
[http://dx.doi.org/10.1016/j.cjche.2017.02.006]
[http://dx.doi.org/10.1016/j.jhazmat.2017.10.009] [PMID: 29055199]
[http://dx.doi.org/10.1016/j.ijbiomac.2018.02.101] [PMID: 29471087]
[http://dx.doi.org/10.1016/j.cej.2017.10.054]
[http://dx.doi.org/10.1039/C7RA06163C]
[http://dx.doi.org/10.1177/0263617417705473]
[http://dx.doi.org/10.1016/j.chemosphere.2016.12.049] [PMID: 28002763]
(b)Ibrahim, S.M.; Noorsal, K.; AIP Conference Proceedings: Advanced Materials for Sustainability and Growth; USA, 2017, pp. 020018-020025.
[http://dx.doi.org/10.1016/j.jece.2017.09.032]
[http://dx.doi.org/10.1080/01496395.2017.1418889]
[http://dx.doi.org/10.1021/acs.jced.6b00827]
[http://dx.doi.org/10.1016/j.biortech.2018.02.019] [PMID: 29454278]
[http://dx.doi.org/10.18520/cs/v113/i12/2282-2291]
[http://dx.doi.org/10.1098/rsos.171927] [PMID: 29657793]
[http://dx.doi.org/10.1016/j.cej.2017.04.095]
[http://dx.doi.org/10.1039/C7NJ04869F]
[http://dx.doi.org/10.1007/s13369-017-2847-x]
[http://dx.doi.org/10.1016/j.physb.2018.02.017]
[http://dx.doi.org/10.1016/j.jhazmat.2012.02.040] [PMID: 22410725]
[http://dx.doi.org/10.1016/j.cej.2010.08.004]
[http://dx.doi.org/10.1016/j.cherd.2016.07.007]
[http://dx.doi.org/10.1016/j.cej.2017.10.148]
[http://dx.doi.org/10.1039/C6NR09638G] [PMID: 28225117]
[http://dx.doi.org/10.1021/es301967y] [PMID: 23050661]
[http://dx.doi.org/10.1128/AEM.63.6.2442-2445.1997] [PMID: 9172366]
[http://dx.doi.org/10.1128/AEM.65.12.5279-5284.1999] [PMID: 10583977]
[http://dx.doi.org/10.1007/s002530100620] [PMID: 11499944]
[http://dx.doi.org/10.1016/j.biortech.2005.08.014] [PMID: 16219462]
[http://dx.doi.org/10.1007/s11705-012-1284-3]
[http://dx.doi.org/10.1016/j.cej.2012.09.074]
[http://dx.doi.org/10.1016/j.jhazmat.2008.02.116] [PMID: 18400378]
[http://dx.doi.org/10.1021/es2018708] [PMID: 22126585]
[http://dx.doi.org/10.1016/j.jhazmat.2010.11.009] [PMID: 21134716]
[http://dx.doi.org/10.1016/j.jhazmat.2005.12.021] [PMID: 16439060]
[http://dx.doi.org/10.1016/S1381-5148(99)00011-5]
[http://dx.doi.org/10.1016/j.cej.2012.06.131]
[http://dx.doi.org/10.1039/C4CS00002A] [PMID: 24831234]
[http://dx.doi.org/10.1039/C2CS35241A] [PMID: 22968228]
[http://dx.doi.org/10.1080/19443994.2015.1012745]
[http://dx.doi.org/10.1007/s13738-017-1190-1]
[http://dx.doi.org/10.1016/j.cej.2013.08.016]
[http://dx.doi.org/10.1016/j.jece.2016.08.001]
[http://dx.doi.org/10.15376/biores.11.3.7145-7161]
[http://dx.doi.org/10.1021/am504896w] [PMID: 25299972]
[http://dx.doi.org/10.1039/C4RA09999K]
[http://dx.doi.org/10.1002/adma.201302400] [PMID: 24108549]
[http://dx.doi.org/10.1021/ja108482a] [PMID: 21142154]
[http://dx.doi.org/10.1016/j.snb.2017.07.149]
[http://dx.doi.org/10.1063/1.5009585] [PMID: 29117701]
[http://dx.doi.org/10.1002/cphc.201300084] [PMID: 23818114]
[http://dx.doi.org/10.1080/19443994.2012.749177]
[http://dx.doi.org/10.1002/ppsc.201200139]
[http://dx.doi.org/10.1007/s13369-017-2438-x]
[http://dx.doi.org/10.1016/j.jhazmat.2017.08.072] [PMID: 28892798]
[http://dx.doi.org/10.1039/C5NJ01348H]
[http://dx.doi.org/10.1021/jacs.7b07123] [PMID: 28782951]
[http://dx.doi.org/10.1016/j.cej.2017.03.015]
[http://dx.doi.org/10.1080/19443994.2015.1065768]
[http://dx.doi.org/10.1080/19443994.2013.815682]